聚合物Janus微粒的合成方法及特性綜述(4),高分子材料論文

聚合物Janus微粒的合成方法及特性綜述(4),高分子材料論文4.5其他應(yīng)用。Synytska等[108]先通過Pickering乳液修飾法制備PAA/PSJanus微粒，然后在PAA端載入Ag和Au納米粒子，得到了具有高界面催化活性的復(fù)合型Janus微粒。復(fù)合型Janus微粒能有效降解亞甲基藍(lán)、曙紅Y和對硝基苯酚，并具有用量少、易回收、可重復(fù)使用等優(yōu)點(diǎn)?；隍蝌叫徒宦?lián)的PMMA-b-P4VP聚合物Janus納米粒子穩(wěn)定的乳液，Gao等[109]簡單合成了宏蜂窩聚合物泡沫材料及載入Pd的高活性雜合泡沫催化劑。除此之外，聚合物Janus微粒還可作為吸附劑[110]和微反響器[111],并能用于制備超疏水涂層[16]等。5結(jié)論。聚合物Janus微粒具有的多功能組分、各向異性外表性質(zhì)和微觀形貌和多種環(huán)境響應(yīng)性使其在外表活性劑和藥物控釋等諸多領(lǐng)域具有獨(dú)特優(yōu)勢。通過合理的設(shè)計(jì)，人們已經(jīng)能夠可控制備具有期望尺寸、性質(zhì)、形貌和組分的聚合物Janus微粒。Pickering乳液修飾法和種子聚合法合適于大量制備亞微米聚合物，是最可能實(shí)現(xiàn)工業(yè)應(yīng)用的方式方法?？煽?活性聚合法和微流體技術(shù)則能夠更好地控制微粒構(gòu)造；自組裝法適于制備納米級的多層級聚合物微粒。當(dāng)前，聚合物Janus微粒的研究主要是合成聚合物。含有天然組分和純天然環(huán)境友好型聚合物Janus材料的制備還較少，其制備和應(yīng)用將會是將來發(fā)展的趨勢之一。其次，怎樣實(shí)現(xiàn)納米級聚合物Janus粒子構(gòu)造的精到準(zhǔn)確控制及大量制備仍然是急需解決的問題。而聚合物構(gòu)造-性質(zhì)-應(yīng)用的互相關(guān)系還需進(jìn)一步研究?？傊?，通過對聚合物Janus微粒改性方式方法的創(chuàng)新，將有助于制備具有新型功能的聚合物Janus材料，并拓寬其應(yīng)用領(lǐng)域。參考文獻(xiàn)：[1]deGennesPG.Angew.Chem.Int.Ed.,1992,31:842.[2]WaltherA,MllerAHE.Chem.Rev.,2020,113:5194.[3]LattuadaM,HattonTA.NanoToday,2018,6:286.[4]Cole-HamiltonDJ.Science,2018,327:41.[5]SchickI,LorenzS,GehrigD,SchilmannAM,BauerH,PanthferM,FischerK,StrandD,LaquaiF,TremelW.J.Am.Chem.Soc.,2020,136:2473.[6]CoxLM,KillgoreJP,LiZ,ZhangZ,HurleyDC,XiaoJ,DingY.Adv.Mater.,2020,26:899.[7]LeeKJ,YoonJ,LahannJ.Curr.Opin.Colloid.In.,2018,16:195.[8]周鵬〔ZhouP〕,劉寶〔LiuB〕,梁福鑫〔LiangFX〕,王倩〔WangQ〕,屈小中〔QuXZ〕,楊振忠〔YangZZ〕.高等學(xué)校化學(xué)學(xué)報(bào)〔ChemicalJournalofChineseUniversities〕,2021,36:1431.[9]LiangF,ZhangC,YangZ.Adv.Mater.,2020,26:6944.[10]PercecV,WilsonDA,LeowanawatP,WilsonCJ,HughesAD,KaucherMS,HammerDA,LevineDH,KimAJ,BatesFS,DavisKP,LodgeTP,KleinML,DeVaneRH,AqadE,RosenBM,ArgintaruAO,SienkowskaMJ,RissanenK,NummelinS,RopponenJ.Science,2018,328:1009.[11]DupontJ,LiuG.SoftMatter,2018,6:3654.[12]WangT,ChenSR,JinF,CaiJH,CuiLY,ZhengYM,WangJX,SongYL,JiangL.Chem.Commun.,2021,51:1367.[13]GhoussoubYE,SchlenoffJB.Langmuir,2021,32:3623.[14]TangC,ZhangC,SunY,LiangF,WangQ,LiJ,QuX,YangZ.Macromolecules,2020,46:188.[15]DengR,LiuS,LiangF,WangK,ZhuJ,YangZ.Macromolecules,2020,47:3701.[16]ZhaoH,LiangF,QuX,WangQ,YangZ.Macromolecules,2021,48:700.[17]YangH,LiangF,ChenY,WangQ,QuX,YangZ.NPGAsiaMater.,2021,7:e176.[18]HuJ,ZhouS,SunY,FangX,WuL.Chem.Soc.Rev.,2020,41:4356.[19]KaewsanehaC,TangboriboonratP,PolpanichD,EissaM,ElaissariA.ACSAppl.Mater.Interfaces,2020,5:1857.[20]KaewsanehaC,TangboriboonratP,PolpanichD,EissaaM,ElaissariA.ColloidsandSurfacesA:Physicochem.Eng.Aspects,2020,439:35.[21]陳云華〔ChenYH〕,王朝陽〔WangCY〕,李煜〔LiY〕,童真〔TongZ〕.化學(xué)進(jìn)展〔ProgressinChemistry〕,2018,21:615.[22]劉善芹〔LiuSQ〕,張毅軍〔ZhangYJ〕,鄧仁華〔DengRH〕,梅路平〔MeiLP〕.科技導(dǎo)報(bào)〔ScienceTechnologyReview〕,2021,34:27.[23]NisisakoT.Curr.Opin.Colloid.In.,2021,25:1.[24]楊軼〔YangY〕,葉偉〔YeW〕,陳曉〔ChenX〕.物理化學(xué)學(xué)報(bào)〔ActaPhysico-ChimicaSinica〕,2020,28:2525.[25]ChoI,LeeKWJ.Appl.Polym.Sci.,1985,30:1903.[26]YabuH,KanaharaM,ShimomuraM,AritaT,HaranoK,NakamuraE,HiguchiT,JinnaiH.ACSAppl.Mater.Interfaces,2020,5:3262.[27]UrbanM,FreisingerB,GhazyO,StaffR,LandfesterK,CrespyD,MusyanovychA.Macromolecules,2020,47:7194.[28]WeissS,HirsemannD,BiersackB,ZiadehM,MllerAHE,BreuJ.Polymer,2020,54:1388.[29]PerroA,ReculusaS,RavaineS,Bourgeat-LamicE,DuguetE.J.Mater.Chem.,2005,15:3745.[30]ZhangJT,ChaoX,AsherSA.J.Am.Chem.Soc.,2020,135:11397[31]PoggiE,BourgeoisJP,ErnouldB,GohyJF.RSCAdv.,2021,5:44218.[32]SeidelP,RavooBJ.Macromol.Chem.Phys.,2021,217:1467.[33]YamagamiT,KitayamaY,OkuboM.Langmuir,2020,30:7823.[34]LiuJ,LiuG,ZhangM,SunP,ZhaoH.Macromolecules,2020,46:5974.[35]HuangC,ShenX.Chem.Commun.,2020,50:2646.[36]SuzukiD,TsujiS,KawaguchiH.J.Am.Chem.Soc.,2007,129:8088.[37]WuH,YiW,ChenZ,WangH,DuQ.Carbon,2021,93:473.1ACSAppl.Mater.Interfaces,2021,7:9744.[39]ChoiCH,WeitzDA,LeeCS.Adv.Mater.,2020,25:2536.[40]CaoX,LiW,MaT,DongH.RSCAdv.,2021,5:79969.[41]SunX,LiuM,XuZ.Talanta,2020,121:163.[42]HuY,WangS,AbbaspourradA,ArdekaniAM.Langmuir,2021,31:1885.[43]MaedaK,OnoeH,TakinoueM,TakeuchiS.Adv.Mater.,2020,24:1340.[44]HuY,WangJ,LiC,WangQ,WangH,ZhuJ,YangY.Langmuir,2020,29:15529.[45]YoonJ,KotaA,BhaskarS,TutejaA,LahannJ.ACSAppl.Mater.Interfaces,2020,5:11281.[46]MisraAC,LukerKE,DurmazH,LukerGD,LahannJ.Biomacromolecules,2021,16:2412.[47]YoonJ,EysterTW,MisraAC,LahannJ.Adv.Mater.,2021,27:4509.[48]JinZ,FanH.SoftMatter,2020,10:9212[49]GrschelAH,MllerAHE.Nanoscale,2021,7:11841.[50]ErhardtR,BkerA,ZettlH,KayaH,Pyckhout-HintzenW,KrauschG,AbetzV,MllerAHE.Macromolecules,2001,34:1069.[51]WaltherA,MllerAHE.SoftMatter,2008,4:663.[52]GrschelAH,SchacherFH,SchmalzH,BorisovOV,ZhulinaEB,WaltherA,MllerAHE.Nat.Commun.,2020,3:710.[53]GrschelAH,WaltherA,LblingTI,SchacherFH,SchmalzH,MllerAHE.Nature,2020,503:247.[54]HiekkataipaleP,LblingTI,PoutanenM,PriimagiA,AbetzV,IkkalaO,GrschelAH.Polymer,2021,DOI:10.1016/j.polymer.2021.05.076.[55]DengRH,LiangFX,ZhouP,ZhangCL,QuXZ,WangQ,ZhuJT,YangZ.Adv.Mater.,2020,26:4469.[56]TranN,MuletX,HawleyAM,ConnCE,ZhaiJ,WaddingtonLJ,DrummondCJ.NanoLett.,2021,15:4229.[57]SkelhonTS,ChenY,BonSAF.Langmuir,2020,3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